Self-assembly is one of the central themes in biologically controlled synthesis, and it also plays a pivotal role in fabricating a variety of advanced engineering materials. In particular, evaporation-induced self-assembly of colloidal particles enables versatile fabrication of highly ordered two- or three-dimensional nanostructures for optical, sensing, catalytic, and other applications. While it is well known that this process results in the formation of the face-centered cubic (fcc) lattice with the close-packed {111} plane parallel to the substrate, the crystallographic texture development of colloidal crystals is less understood. In this study, we show that the preferred <110> growth in the fcc colloidal crystals synthesized through evaporation-induced assembly is achieved through a gradual crystallographic rotation facilitated by mechanical stress-induced geometrically necessary dislocations.
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Song, Yongli ; Guerrero-Juarez, Christian F. ; Chen, Zhongjian ; Tang, Yichen ; Ma, Xianghui ; Lv, Cong ; Bi, Xueyun ; Deng, Min ; Bu, Lina ; Tian, Yuhua ; et al ( , Cell Research)null (Ed.)